All Faculty and Research Staff Publications

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2010
Izawa Y, Stahl SS. Aerobic Oxidative Coupling of o-Xylene: Discovery of 2-Fluoropyridine as a Ligand to Support Selective Pd-Catalyzed C-H Functionalization. Advanced Synthesis & Catalysis. 2010 ;352:3223-3229.
Campbell AN, White PB, Guzei IA, Stahl SS. Allylic C-H Acetoxylation with a 4,5-Diazafluorenone-Ligated Palladium Catalyst: A Ligand-Based Strategy To Achieve Aerobic Catalytic Turnover. Journal of the American Chemical Society. 2010 ;132:15116-15119.
Dohm MT, Mowery BP, Czyzewski AM, Stahl SS, Gellman SH, Barron AE. Biophysical Mimicry of Lung Surfactant Protein B by Random Nylon-3 Copolymers. Journal of the American Chemical Society. 2010 ;132:7957-7967.
King AE, Huffman LM, Casitas A, Costas M, Ribas X, Stahl SS. Copper-Catalyzed Aerobic Oxidative Functionalization of an Arene C-H Bond: Evidence for an Aryl-Copper(III) Intermediate. Journal of the American Chemical Society. 2010 ;132:12068-12073.
Ye X, Johnson MD, Diao T, Yates MH, Stahl SS. Development of safe and scalable continuous-flow methods for palladium-catalyzed aerobic oxidation reactions. Green Chemistry. 2010 ;12:1180-1186.
Casitas A, King AE, Parella T, Costas M, Stahl SS, Ribas X. Direct observation of Cu-I/Cu-III redox steps relevant to Ullmann-type coupling reactions. Chemical Science. 2010 ;1:326-330.
Popp BV, Morales CM, Landis CR, Stahl SS. Electronic Structural Comparison of the Reactions of Dioxygen and Alkenes with Nitrogen-Chelated Palladium(0). Inorganic Chemistry. 2010 ;49:8200-8207.
McDonald RI, Wong GW, Neupane RP, Stahl SS, Landis CR. Enantioselective Hydroformylation of N-Vinyl Carboxamides, Allyl Carbamates, and Allyl Ethers Using Chiral Diazaphospholane Ligands. Journal of the American Chemical Society. 2010 ;132:14027-14029.
Gerken JB, Landis EC, Hamers RJ, Stahl SS. Fluoride-Modulated Cobalt Catalysts for Electrochemical Oxidation of Water under Non-Alkaline Conditions. Chemsuschem. 2010 ;3:1176-1179.
Zhang J, Gellman SH, Stahl SS. Kinetics of Anionic Ring-Opening Polymerization of Variously Substituted beta-Lactams: Homopolymerization and Copolymerization. Macromolecules. 2010 ;43:5618-5626.
McDonald RI, Stahl SS. Modular Synthesis of 1,2-Diamine Derivatives by Palladium-Catalyzed Aerobic Oxidative Cyclization of Allylic Sulfamides. Angewandte Chemie-International Edition. 2010 ;49:5529-5532.
Casitas A, Poater A, Sola M, Stahl SS, Costas M, Ribas X. Molecular mechanism of acid-triggered aryl-halide reductive elimination in well-defined aryl-Cu-III-halide species. Dalton Transactions. 2010 ;39:10458-10463.
Stahl SS. Organotransition Metal Chemistry: From Bonding to Catalysis by John Hartwig.; 2010 pp. 8524-8525.
2009
Zhang JH, Kissounko DA, Lee SE, Gellman SH, Stahl SS. Access to Poly-beta-Peptides with Functionalized Side Chains and End Groups via Controlled Ring-Opening Polymerization of beta-Lactams. Journal of the American Chemical Society. 2009 ;131:1589-1597.
Stephenson NA, Zhu J, Gellman SH, Stahl SS. Catalytic Transamidation Reactions Compatible with Tertiary Amide Metathesis under Ambient Conditions. Journal of the American Chemical Society. 2009 ;131:10003-10008.
Popp BV, Stahl SS. Mechanism of Pd(OAc)(2)/Pyridine Catalyst Reoxidation by O-2: Influence of Labile Monodentate Ligands and Identification of a Biomimetic Mechanism for O-2 Activation. Chemistry-A European Journal. 2009 ;15:2915-2922.
King AE, Brunold TC, Stahl SS. Mechanistic Study of Copper-Catalyzed Aerobic Oxidative Coupling of Arylboronic Esters and Methanol: Insights into an Organometallic Oxidase Reaction. Journal of the American Chemical Society. 2009 ;131:5044-+.
Lee M-R, Stahl SS, Gellman SH, Masters KS. Nylon-3 Copolymers that Generate Cell-Adhesive Surfaces Identified by Library Screening. Journal of the American Chemical Society. 2009 ;131:16779-16789.
Yang LJ, Lu Z, Stahl SS. Regioselective copper-catalyzed chlorination and bromination of arenes with O-2 as the oxidant. Chemical Communications. 2009 :6460-6462.
Scarborough CC, McDonald RI, Hartmann C, Sazama GT, Bergant A, Stahl SS. Steric Modulation of Chiral Biaryl Diamines via Pd-Catalyzed Directed C-H Arylation. Journal of Organic Chemistry. 2009 ;74:2613-2615.
Mowery BP, Lindner AH, Weisblum B, Stahl SS, Gellman SH. Structure-activity Relationships among Random Nylon-3 Copolymers That Mimic Antibacterial Host-Defense Peptides. Journal of the American Chemical Society. 2009 ;131:9735-9745.
Scarborough CC, Bergant A, Sazama GT, Guzei IA, Spencer LC, Stahl SS. Synthesis of Pd-II complexes bearing an enantiomerically resolved seven-membered N-heterocyclic carbene ligand and initial studies of their use in asymmetric Wacker-type oxidative cyclization reactions. Tetrahedron. 2009 ;65:5084-5092.
2008
Huffman LM, Stahl SS. Carbon-nitrogen bond formation involving well-defined aryl-copper(III) complexes. Journal of the American Chemical Society. 2008 ;130:9196-+.
Hamada T, Ye X, Stahl SS. Copper-catalyzed aerobic oxidative amidation of terminal alkynes: Efficient synthesis of ynamides. Journal of the American Chemical Society. 2008 ;130:833-+.
Hoerter JM, Otte KM, Gellman SH, Cui Q, Stahl SS. Discovery and mechanistic study of Al-III-catalyzed transamidation of tertiary amides. Journal of the American Chemical Society. 2008 ;130:647-654.
Epand RF, Mowery BP, Lee SE, Stahl SS, Lehrer RI, Gellman SH, Epand RM. Dual mechanism of bacterial lethality for a cationic sequence-random copolymer that mimics host-defense antimicrobial peptides. Journal of Molecular Biology. 2008 ;379:38-50.
Hewgley BJ, Stahl SS, Kozlowski MC. Mechanistic study of asymmetric oxidative biaryl coupling: Evidence for self-processing of the copper catalyst to achieve control of oxidase vs oxygenase activity. Journal of the American Chemical Society. 2008 ;130:12232-+.
Konnick MM, Stahl SS. Reaction of molecular oxygen with a Pd-II-hydride to produce a Pd-II-hydroperoxide: Experimental evidence for an HX-reductive-elimination pathway. Journal of the American Chemical Society. 2008 ;130:5753-5762.
Lee MR, Stahl SS, Gellman SH. Synthesis of beta-Lactams Bearing Functionalized Side Chains from a Readily Available Precursor. Organic Letters. 2008 ;10:5317-5319.
2007
Bell CM, Kissounko DA, Gellman SH, Stahl SS. Catalytic metathesis of simple secondary amides. Angewandte Chemie-International Edition. 2007 ;46:761-763.
Popp BV, Stahl SS. Insertion of Molecular Oxygen into a Palladium-Hydride Bond: Computational Evidence for Two Nearly Isoenergetic Pathways. Journal of the American Chemical Society. 2007 ;129:4410-4422.
Mowery BP, Lee SE, Kissounko DA, Epand RF, Epand RM, Weisblum B, Stahl SS, Gellman SH. Mimicry of antimicrobial host-defense peptides by random copolymers. Journal of the American Chemical Society. 2007 ;129:15474-15476.
Kotov V, Scarborough CC, Stahl SS. Palladium-catalyzed aerobic oxidative amination of alkenes: Development of intra- and intermolecular Aza-Wacker reactions. Inorganic Chemistry. 2007 ;46:1910-1923.
Rogers MM, Kotov V, Chatwichien J, Stahl SS. Palladium-Catalyzed Oxidative Amination of Alkenes: Improved Catalyst Reoxidation Enables the Use of Alkene as the Limiting Reagent. Organic Letters. 2007 ;9:4331-4334.
Popp BV, Wendlandt JE, Landis CR, Stahl SS. Reaction of molecular oxygen with an NHC-coordinated Pd-0 complex: Computational insights and experimental implications. Angewandte Chemie-International Edition. 2007 ;46:601-604.
Kissounko DA, Hoerter JM, Guzei IA, Cui Q, Gellman SH, Stahl SS. Ti-IV-mediated reactions between primary amines and secondary carboxamides: Amidine formation versus transamidation. Journal of the American Chemical Society. 2007 ;129:1776-1783.
Liu G, Stahl SS. Two-faced reactivity of alkenes: cis- versus trans-aminopalladation in aerobic pd-catalyzed intramolecular Aza-Wacker reactions. Journal of the American Chemical Society. 2007 ;129:6328-6335.
2006
Rogers MM, Wendlandt JE, Guzei IA, Stahl SS. Aerobic intramolecular oxidative amination of alkenes catalyzed by NHC-coordinated palladium complexes. Organic Letters. 2006 ;8:2257-2260.
Liu G, Stahl SS. Highly regioselective Pd-catalyzed intermolecular aminoacetoxylation of alkenes and evidence for cis-aminopalladation and S(N)2 C-O bond formation. Journal of the American Chemical Society. 2006 ;128:7179-7181.
Hoerter JM, Otte KM, Gellman SH, Stahl SS. Mechanism of Al-III-catalyzed transamidation of unactivated secondary carboxamides. Journal of the American Chemical Society. 2006 ;128:5177-5183.
Steinhoff BA, Stahl SS. Mechanism of Pd(OAc)(2)/DMSO-catalyzed aerobic alcohol oxidation: Mass-transfer-limitation effects and catalyst decomposition pathways. Journal of the American Chemical Society. 2006 ;128:4348-4355.
Popp BV, Stahl SS. "Oxidatively induced" reductive elimination of dioxygen from an eta(2-) peroxopalladium(II) complex promoted by electron-deficient alkenes. Journal of the American Chemical Society. 2006 ;128:2804-2805.
Konnick MM, Gandhi BA, Guzei IA, Stahl SS. Reaction of molecular oxygen with a Pd-II-hydride to produce a Pd-II-hydroperoxide: Acid catalysis and implications for Pd-catalyzed aerobic oxidation reactions. Angewandte Chemie-International Edition. 2006 ;45:2904-2907.
Popp BV, Thorman JL, Stahl SS. Similarities between the reactions of dioxygen and alkenes with palladium(0): Relevance to the use of benzoquinone and molecular oxygen as stoichiometric oxidants in palladium-catalyzed oxidation reactions. Journal of Molecular Catalysis A. 2006 ;251:2-7.
Scarborough CC, Stahl SS. Synthesis of pyrrolidines via palladium(II)-catalyzed aerobic oxidative carboamination of butyl vinyl ether and styrenes with allyl tosylamides. Organic Letters. 2006 ;8:3251-3254.
Steinhoff BA, King AE, Stahl SS. Unexpected roles of molecular sieves in palladium-catalyzed aerobic alcohol oxidation. Journal of Organic Chemistry. 2006 ;71:1861-1868.

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